By Pietro Chiodi
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Strey. J. Chem. Phys. 2010, 132, 064304 13. Oxtoby, D. W. J. Chem. Phys. 1988, 89, 7521. 14. Pan, A. , and D. Chandler. J. Phys. Chem. B 2004, 108, 19681. 15. ten Wolde, P. , and D. Frenkel. J. Chem. Phys. 1998, 109, 9901. 16. , S. Chakrabarty, and B. Bagchi. J. Chem. Phys. 2008, 129, 234704. 17. , D. Donadio, and M. Parrinello. Phys. Rev. Lett. 2006, 97, 105701. (a) Davis, M. , and R. F. Lobo. Chem. Mater. 1992, 4, 756. , A. Navrotsky, M. E. Davis, and S. I. Zones. Chem. Mater. 1993, 5, 1805.
CNT assumes that a spherical droplet of the new stable phase grows in a sea of parent metastable bulk phase by addition of single molecules and that this droplet has to grow beyond a certain “critical size” (R*) to compensate for the energy required to form the surface between the two phases. 1) 3 where │ΔGV│ is the free energy difference per unit volume between the daughter and the parent phases, and γ is the surface tension of the interface between them. 2) 3(∆GV )2 Note that the free energy barrier depends more strongly on surface tension than on the free energy difference.
Is there a particular incident from your research career, an anecdote, that you would like to share with the readers? I recall an incident which helped to redefine the course of my research. Around 1970, I had written an article on what I called “the force concept in chemistry” for students and teachers of chemistry. The chemistry journals I sent it to declined to consider it for publication, saying this would be beyond their readership. Exasperated, I sent it to Professor Coulson for his critical comments.