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Chem. Phys. and R. T. Pack, 92, 810 (1990). J. Phys. Chem. 94, 8055 (1990). [22] S. Takada, A. Ohsaki, [23] S. Sift and H. Rabitz, and H. Nakamura, J. Chem. PIvs. J. Chem. Phys. 86, 6190 (1987). 96, 339 (1992). 6. CONCLUDING REMARKS [24] A. J. C. Verandas, Chem. Phys. 39 F. B. Brown, C. A. Mead, D. G. Truhlar, 86, 6258 (1987). [25] J. Z. H. Zhang and W. H. Miller, " and N. C. Blais, J. [26] The S-matrix version the field of nuclear J. Chem. Phys. of the Kohn variational physics; 91, 1528 (1989).

60] performed representation grid over an infinite significant wavepacket to augment grid over a finite interval, volves a uniform whether system. FUNCTION grid points The uniform in reactive includes and Wyatt many improvements is a uniform small. functions GREEN'S by deleting is vanishingly of potential years ago on the H+H2 incorporated SERIES in this DVR has demonstrated basic component. twenty POWER of the potential function the gross anharmonicity Thus, 3. of the time evolution operator.

Chu, and W. H. Miller, J. Chem. Phys. 88, 6233 (1988). [23] D. E. Manolopoulos and R. E. Wyatt, J. Chem. Phys. 91, 6096 (1989). [24] K. Haug, D. W. Schwenke, Y. Skima, D. G. Truhlar, J. Z. H. Zhang, and D. J. Kouri, J. Phys. Chem. 90, 6757 (1986). [25] For a recent review of this work, see . H. Miller, Annu. Rev. Phys. Chem. 41,245 [26] E. N. Economou, Green's Functions (1990). in Quantum, Physics (Springer, Berlin, 1990). , ........... _ ...................................................................................

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